PhD: AI-assisted discovery of chiral perovskites in structured photonic environment

Job Description

You will leverage an AI-assisted materials optimization robot being developed at AMOLF as a route to rapid, closed-loop synthesis and characterization across large perovskite parameter spaces. You will optimize directly for figures of merit such as chirality, emission wavelength, brightness, and stability. Because optical excitation of perovskites can move atoms around, sculpting the optical field in time and space can enable programmable optical functions. By conducting approximately 1 million optical experiments in parallel using a spatial light modulator and hyperspectral camera, you will explore chemical and processing landscapes in days that would otherwise take a student a lifetime to cover systematically. Special attention will be paid to 2D and related low-dimensional perovskites, with the aim to understand if intrinsically strong material chirality is a necessary condition for reaching strong programmable chirality.

Materials discovery in non-trivial optical environments

Building on the first thrust, you will introduce a new paradigm in optoelectronic device design: to synthesize and screen perovskite emitters directly on substrates that already provide a structured optical response. In a material that can be sculpted by the optical field, this provides the opportunity for a self-optimizing response - the local optical field imprints a symmetry on the material, which then amplifies the light-matter coupling. In the conventional workflow, one first finds a material with good intrinsic properties and only then designs the surrounding cavity, resonance, or metasurface. You will reverse that order, replacing an optically inert glass slide by a substrate with a designed resonance arising from refractive-index structuring (optical metasurface). Thin perovskite films spun onto such a substrate will respond most strongly when their emission (absorption) spectrum aligns with the photonic resonance. Likewise, if the figure of merit is chirality and the substrate itself has chiral optical response, one can search for materials whose intrinsic emission (absorption) couples most effectively to that environment. In this way, the optical structure of the substrate transforms the material on top into exactly what it needs for maximal performance. Such exploration offers tantalizing opportunities to study the impact of local versus nonlocal optical resonances in the context of material optimization. How does the spatial extent of the photonic resonance affect the material symmetry? Does the optical field profile induce spatially varying chiral properties in the perovskite? Understanding the coupling between photonic environment and material crystallization poses completely new opportunities in material synthesis for advanced photonic integration and technologies.

Qualifications

You have a Msc degree in physics, chemistry, materials science, engineering or another scientific discipline. You have an analytical mind with the ability to think about a problem and come up with logical and creative solutions. You can work independently and also enjoy collaborating in a team. You enjoy actively engaging others to learn new concepts and experimental methods. You are eager to give and receive feedback and see it as an opportunity for personal and professional growth. You have excellent communication skills in English. You are responsible, reliable and dedicated while caring about the well-being of yourself and your colleagues. You value and cherish diversity of background, opinion and ability and see a team as more than the sum of its parts.

Work environment

This is a collaborative project between AMOLF and the University of Amsterdam. Your contract and host group will be the Nanoscale Solar Cells group led by Erik Garnett at AMOLF but you will also work part time at the Van der Waals-Zeeman institute of the University of Amsterdam with professors Sander Mann and Jorik van de Groep in the department of physics. These institutes are located next to each other in the Amsterdam Science Park. This collaborative position opens up many experimental and theoretical tools and facilities needed for the project including the AI-assisted automated synthesis and characterization robot, the AMOLF nanolab, ultrafast, chiral and single photon microscopes and full-wave numerical simulations and analytical models. We share a vibrant, inclusive and collaborative work culture that welcomes scientists and engineers with diverse backgrounds and skills. There is a very active staff association organizing regular social activities throughout the year to enrich the work experience and community. There is excellent support staff to help with the more technical and administrative parts of the project.

Working conditions

• The working atmosphere at the institute is largely determined by young, enthusiastic, mostly foreign employees. Communication is informal and runs through short lines of communication.
• The position is intended as full-time (40 hours / week, 12 months / year) appointment in the service of the Netherlands Foundation of Scientific Research Institutes (NWO-I) for the duration of four years
• The starting salary is 3.115 Euro's gross per month and a range of employment benefits.
• After successful completion of the PhD research a PhD degree will be granted at a Dutch University.
• Several courses are offered, specially developed for PhD-students.
• AMOLF assists any new foreign PhD-student with housing and visa applications and compensates their transport costs and furnishing expenses.

More information?

For further information about the position or specific questions, please contact Erik Garnett: [email protected]

Application

You can respond to this vacancy online via the button below. Please apply by submitting a CV and cover letter explaining why you want this specific PhD position, what you can contribute and what you would like to learn. We will start evaluating applications on June 15th and will continue until the position is filled.

Online screening may be part of the selection.

Diversity code

AMOLF is highly committed to an inclusive and diverse work environment: we want to develop talent and creativity by bringing together people from different backgrounds and cultures. We recruit and select on the basis of competencies and talents. We strongly encourage anyone with the right qualifications to apply for the vacancy, regardless of age, gender, origin, sexual orientation or physical ability.

AMOLF has won the NNV Diversity Award 2022, which is awarded every two years by the Netherlands Physical Society for demonstrating the most successful implementation of equality, diversity and inclusion (EDI).

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